Most electrical modules for automotive use are specified for around 9 - 16 V. I don't know what voltage range you will be working to, but you should include voltages well below 12 V so that the lights will work with battery that isn't fully charged.
The Cree XHP70.3 are rated at a maximum of 3600 mA but a lot of their specification are quoted for 1050 mA. For reliability, efficiency and lifetime reasons, I would suggest running them at 1050 mA, although you will need more LEDs to get the same light output.
However, you really don't have enough voltage to run the 12 V ones. They are rated at 11.2 - 12.2 V at 1050 mA. Like most LEDS, they need to be run from a constant current supply, and the voltages are only mentioned so that the constant current supply can be specified to cope with the voltage and if you happen to get LEDs that are near to 12.2 V, they will be dimmer if the battery isn't charged. 12 V LEDs will go out completely when the engine is cranking if you are running from the starter battery.
You should use the 6 V version, with a constant current regulator for each LED. Do not put the LEDs in parallel, as the current may not be shared equally.
You could use three LEDs rated at 3 V each, in series, with a single constant current regulator. That would be more efficient.
Make sure that your regulators can handle the heating at the maximum alternator voltage. You should also consider what happens if an LED shorts out, or partially shorts out. The 6 V LEDs are actually two 3 V LEDs in series, so it's possible for one to be shorted and the other to remain illuminated. You need to make sure that the regulators won't be damaged or overheat something else when there is a short or a partial short, either of which would cause increased heating in a constant current regulator.