yes that's a bit too far,
The 600KHz max frequency is because above that, and you tend to violate the minimum on or off times of the fet. Also, at that higher frequency, the di/dt tends to get higher and the comparator delay becomes more significant and causes led current inaccuracy.
..... even fewer if you use a single hysteretic comparator . For amusement, here's a sim of the twin-comparator and single-comparator versions side by side. Virtually identical LED current profiles can be achieved with component values as shown.
The single can be made to run faster than the twin (by reducing the hysteresis), because of less inherent delay, enabling use of a lower inductance value for a given ripple amount.